Title | Electrically Pumped Polarized Exciton-Polaritons in a Halide Perovskite Microcavity |
Authors | Wang, Tingting Zang, Zhihao Gao, Yuchen Lyu, Chao Gu, Pingfan Yao, Yige Peng, Kai Watanabe, Kenji Taniguchi, Takashi Liu, Xiaoze Gao, Yunan Bao, Wei Ye, Yu |
Affiliation | Peking Univ, State Key Lab Mesoscop Phys, Sch Phys, Beijing 100871, Peoples R China Peking Univ, Frontiers Sci Ctr Nanooptoelect, Sch Phys, Beijing 100871, Peoples R China Collaborat Innovat Ctr Quantum Matter, Beijing 100871, Peoples R China Natl Inst Mat Sci, Res Ctr Funct Mat, Tsukuba, Ibaraki 3050044, Japan Natl Inst Mat Sci, Int Ctr Mat Nanoarchitecton, Tsukuba, Ibaraki 3050044, Japan Wuhan Univ, Sch Phys & Technol, Wuhan 430072, Hubei, Peoples R China Wuhan Inst Quantum Technol, Wuhan 430206, Hubei, Peoples R China Univ Nebraska, Elect & Comp Engn, Lincoln, NE 68588 USA Peking Univ, Yangtze Delta Inst Optoelect, Nantong 226010, Jiangsu, Peoples R China |
Keywords | NANOCRYSTALS ADHESION |
Issue Date | Jun-2022 |
Publisher | NANO LETTERS |
Abstract | Recently, exciton-polaritons in lead halide perovskite microcavities have been extensively investigated to address striking phenomena such as polariton condensation and quantum emulation. However, a critical step in advancing these findings into practical applications, i.e., realizing electrically pumped perovskite polariton light-emitting devices, has not yet been presented. Here, we devise a new method to combine the device with a microcavity and report the first halide perovskite polariton light-emitting device. Specifically, the device is based on a CsPbBr3 capacitive structure, which can inject the electrons and holes from the same electrode, conducive to the formation of excitons and simultaneously maintaining the high quality of the microcavity. In addition, highly polarized polariton emissions have been demonstrated due to the optical birefringence in the CsPbBr3 microplate. This work paves the way for realizing practical polaritonic devices such as high-speed light-emitting devices for information communications and inversionless electrically pumped lasers based on perovskites. |
URI | http://hdl.handle.net/20.500.11897/648724 |
ISSN | 1530-6984 |
DOI | 10.1021/acs.nanolett.2c00906 |
Indexed | SCI(E) |
Appears in Collections: | 物理学院 人工微结构和介观物理国家重点实验室 |