Title Electrically Pumped Polarized Exciton-Polaritons in a Halide Perovskite Microcavity
Authors Wang, Tingting
Zang, Zhihao
Gao, Yuchen
Lyu, Chao
Gu, Pingfan
Yao, Yige
Peng, Kai
Watanabe, Kenji
Taniguchi, Takashi
Liu, Xiaoze
Gao, Yunan
Bao, Wei
Ye, Yu
Affiliation Peking Univ, State Key Lab Mesoscop Phys, Sch Phys, Beijing 100871, Peoples R China
Peking Univ, Frontiers Sci Ctr Nanooptoelect, Sch Phys, Beijing 100871, Peoples R China
Collaborat Innovat Ctr Quantum Matter, Beijing 100871, Peoples R China
Natl Inst Mat Sci, Res Ctr Funct Mat, Tsukuba, Ibaraki 3050044, Japan
Natl Inst Mat Sci, Int Ctr Mat Nanoarchitecton, Tsukuba, Ibaraki 3050044, Japan
Wuhan Univ, Sch Phys & Technol, Wuhan 430072, Hubei, Peoples R China
Wuhan Inst Quantum Technol, Wuhan 430206, Hubei, Peoples R China
Univ Nebraska, Elect & Comp Engn, Lincoln, NE 68588 USA
Peking Univ, Yangtze Delta Inst Optoelect, Nantong 226010, Jiangsu, Peoples R China
Keywords NANOCRYSTALS
ADHESION
Issue Date Jun-2022
Publisher NANO LETTERS
Abstract Recently, exciton-polaritons in lead halide perovskite microcavities have been extensively investigated to address striking phenomena such as polariton condensation and quantum emulation. However, a critical step in advancing these findings into practical applications, i.e., realizing electrically pumped perovskite polariton light-emitting devices, has not yet been presented. Here, we devise a new method to combine the device with a microcavity and report the first halide perovskite polariton light-emitting device. Specifically, the device is based on a CsPbBr3 capacitive structure, which can inject the electrons and holes from the same electrode, conducive to the formation of excitons and simultaneously maintaining the high quality of the microcavity. In addition, highly polarized polariton emissions have been demonstrated due to the optical birefringence in the CsPbBr3 microplate. This work paves the way for realizing practical polaritonic devices such as high-speed light-emitting devices for information communications and inversionless electrically pumped lasers based on perovskites.
URI http://hdl.handle.net/20.500.11897/648724
ISSN 1530-6984
DOI 10.1021/acs.nanolett.2c00906
Indexed SCI(E)
Appears in Collections: 物理学院
人工微结构和介观物理国家重点实验室

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