Title Considerable Unaccounted Local Sources of NO(x)Emissions in China Revealed from Satellite
Authors Kong, Hao
Lin, Jintai
Chen, Lulu
Zhang, Yuhang
Yan, Yingying
Liu, Mengyao
Ni, Ruijing
Liu, Zehui
Weng, Hongjian
Affiliation Peking Univ, Sch Phys, Dept Atmospher & Ocean Sci, Lab Climate & Ocean Atmosphere Studies, Beijing 100871, Peoples R China
China Univ Geosci Wuhan, Sch Environm Sci, Dept Atmospher Sci, Wuhan 430074, Peoples R China
Royal Netherlands Meteorol Inst, R&D Satellite Observat Dept, NL-3731 GA De Bilt, Netherlands
Keywords TROPOSPHERIC NITROGEN-DIOXIDE
NOX EMISSIONS
ANTHROPOGENIC EMISSIONS
SURFACE REFLECTANCE
POWER-PLANTS
AIR-QUALITY
EAST-ASIA
RESOLUTION
OXIDES
UNCERTAINTIES
Issue Date 7-Jun-2022
Publisher ENVIRONMENTAL SCIENCE & TECHNOLOGY
Abstract High-resolution (e.g., 5 km) emission data of nitrogenoxides (NOx=NO+NO2) provide localized knowledge of pollutionsources for targeted regulations, yet such data are lacking or inaccurate overmost regions at present. Here we improve our PHLET-based inversionmethod to derive NOxemissions in China at a 5-km resolution in summer2019, based on the TROPOMI-POMINO satellite product of nitrogendioxide (NO2) columns. With low computational costs, our inversionexplicitly accounts for the effects of horizontal transport and nonlinearchemistry. Wefind numerous small-to-medium sources related to minorroads and small human settlements at relatively low affluence levels, inaddition to clear emission signals along major transportation lines,consistent with road line density and Tencent location data. Many small-to-medium sources and transportation emissions are unclear or missing inthe spatial distributions of four widely used emission inventories. Our emissions offer a unique reference for targeted emissioncontrol.
URI http://hdl.handle.net/20.500.11897/647925
ISSN 0013-936X
DOI 10.1021/acs.est.1c07723
Indexed SCI(E)
Appears in Collections: 物理学院

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