Title Modeling of Flame Retardants in Typical Urban Indoor Environments in China during 2010-2030: Influence of Policy and Decoration and Implications for Human Exposure
Authors Li, Zengwei
Zhu, Ying
Wang, Dou
Zhang, Xianming
Jones, Kevin C.
Ma, Jianmin
Wang, Pu
Yang, Ruiqiang
Li, Yingming
Pei, Zhiguo
Zhang, Qinghua
Jiang, Guibin
Affiliation Chinese Acad Sci, Res Ctr Ecoenvironm Sci, State Key Lab Environm Chem & Ecotoxicol, Beijing 100085, Peoples R China
Univ Chinese Acad Sci, Beijing 100049, Peoples R China
Zhejiang Acad Agr Sci, Inst Qual & Stand Agroprod, Lab Hangzhou Risk Assessment Agr Prod, Minist Agr, Hangzhou 310021, Zhejiang, Peoples R China
Concordia Univ, Dept Chem & Biochem, West Montreal, PQ H4B 1R6, Canada
Univ Lancaster, Lancaster Environm Ctr, Lancaster LA1 4YQ, England
Peking Univ, Coll Urban & Environm Sci, Lab Earth Surface Proc, Beijing 100871, Peoples R China
Shanghai Jiao Tong Univ, Sch Environm Sci & Engn, Shanghai 200240, Peoples R China
Keywords POLYBROMINATED DIPHENYL ETHERS
HUMAN DIETARY EXPOSURE
CONSUMER PRODUCTS
DIFFERENT MICROENVIRONMENTS
ORGANIC-COMPOUNDS
ORGANOPHOSPHATE
DUST
AIR
PBDES
EMISSIONS
Issue Date 7-Sep-2021
Publisher ENVIRONMENTAL SCIENCE & TECHNOLOGY
Abstract Novel flame retardants (FRs) are of increasing concern, given growing evidence of health effects and use to replace polybrominated diphenyl ethers (PBDEs). This study modeled combined effects of use policies and decoration on indoor FRs and human exposure for 18 widely used PBDEs, organophosphate esters (OPEs), and novel brominated flame retardants in typical urban indoor environments in China. The current estimated indoor emission rates and average concentrations in air and dust of the 18 FRs were 10(2)-10(3) ng/h, 561 ng/m(3), and 1.5 x 10(4) ng/g, respectively, with seven OPEs dominant (>69%). Different use patterns exist between China and the US and Europe. Scenarios modeled over 2010-2030 suggested that decoration would affect indoor concentrations of FRs more than use policies, and use policies were mainly responsible for shifts of FR composition. Additional use of hexabromobenzene and 2,3,4,5,6-pentabromotoluene and removal of BDE-209 would make the total human exposure to the modeled FR mixture increase after the restriction of penta- and octa-BDE but decrease after deca-BDE was banned. Better knowledge of the toxicity of substitutes is needed for a complete understanding of the health implications of such changes. Toddlers may be more affected by use changes than adults. Such studies are supportive to the management of FR use.Y
URI http://hdl.handle.net/20.500.11897/624619
ISSN 0013-936X
DOI 10.1021/acs.est.1c03402
Indexed SCI(E)
Appears in Collections: 城市与环境学院
地表过程分析与模拟教育部重点实验室

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