Title Organic-inorganic hybrid perovskite for low-cost and high-performance xerographic photoreceptors
Authors Gu, Wei-Min
Wang, Chuanxi
Gao, Cai-Yan
Fan, Xin-Heng
Yang, Lian-Ming
Jiang, Ke-Jian
Affiliation Chinese Acad Sci, Inst Chem, Key Lab Green Printing, Beijing 100190, Peoples R China
Univ Chinese Acad Sci, Beijing 100190, Peoples R China
Peking Univ, Coll Chem & Mol Engn, Beijing Natl Lab Mol Sci BNLMS, State Key Lab Struct Chem Unstable & Stable Speci, Beijing 100190, Peoples R China
Keywords ION MIGRATION
ELECTRONIC-PROPERTIES
SQUARAINE CHEMISTRY
SOLAR-CELLS
PHTHALOCYANINE
STABILITY
EFFICIENT
Issue Date 30-Jun-2021
Publisher RSC ADVANCES
Abstract Solution-processable organic-inorganic hybrid perovskites are being widely investigated for many applications, including solar cells, light-emitting diodes, photodetectors, and lasers. Herein, we report, for the first time, successful fabrication of xerographic photoreceptors using methylammonium lead iodide (CH3NH3PbI3) perovskite as a light-absorbing material. With the incorporation of polyethylene glycol (PEG) into the perovskite film, the ion migration inherent to the perovskite material can be effectively suppressed, and the resulting photoreceptor exhibits a high and panchromatic photosensitivity, large surface potential, low dark decay, and high environmental resistance and electrical cycling stability. Specifically, the energies required to photodischarge one half of the initial surface potential (E-0.5) are 0.074 mu J cm(-2) at 550 nm and 0.14 mu J cm(-2) at 780 nm, respectively. The photosensitivites outmatch those of the conventionally used organic pigments having narrow spectral responses. Our findings inform a new generation of highly efficient and low-cost xerographic photoreceptors based on perovskite materials.
URI http://hdl.handle.net/20.500.11897/618279
DOI 10.1039/d1ra02717d
Indexed SCI(E)
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