Title Dislocation-induced large local polarization inhomogeneity of ferroelectric materials
Authors Li, Ning
Zhu, Ruixue
Cheng, Xiaoxing
Liu, Heng-Jui
Zhang, Zhangyuan
Huang, Yen-Lin
Chu, Ying-Hao
Chen, Long-Qing
Ikuhara, Yuichi
Gao, Peng
Affiliation Peking Univ, Int Ctr Quantum Mat, Beijing 100871, Peoples R China
Peking Univ, Electron Microscopy Lab, Sch Phys, Beijing 100871, Peoples R China
Penn State Univ, Dept Mat Sci & Engn, University Pk, PA 16802 USA
Natl Chung Hsing Univ, Dept Mat Sci & Engn, Taichung 40227, Taiwan
Natl Chiao Tung Univ, Dept Mat Sci & Engn, Hsinchu 30010, Taiwan
Acad Sinica, Inst Phys, Taipei 11529, Taiwan
Univ Tokyo, Inst Engn Innovat, Tokyo 1138656, Japan
Collaborat Innovat Ctr Quantum Matter, Beijing 100871, Peoples R China
Issue Date 15-Mar-2021
Publisher SCRIPTA MATERIALIA
Abstract Dislocations in ferroelectrics play important roles in ferroelectricity, piezoelectricity, and dielectricity. However, the intrinsic charge-lattice coupling mechanism in ferroelectric crystals containing dislocations is still not well understood. Here, we report a large local polarization inhomogeneity of similar to 100 mu Ccm(-2) induced by a single a[001] dislocation in the PbZr0.2Ti0.8O3/SrTiO3 film/substrate heterostructure, the tensile region (similar to 120 mu Ccm(-2)) and the compressive strain region (similar to 21 mu Ccm(-2)) around the dislocation forms a butterfly-like area. This study reveals the dramatic effects of dislocations on local polarization and provides a strategy to manipulate the polarization magnitude and orientation of local polarization by defect engineering. (C) 2020 Acta Materialia Inc. Published by Elsevier Ltd. All rights reserved.
URI http://hdl.handle.net/20.500.11897/610365
ISSN 1359-6462
DOI 10.1016/j.scriptamat.2020.11.009
Indexed SCI(E)
Appears in Collections: 量子材料科学中心
物理学院

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