Title Doping-dependent phonon anomaly and charge-order phenomena in the HgBa2CuO4+delta and HgBa2CaCu2O6+delta superconductors
Authors Wang, Lichen
Yu, Biqiong
Jing, Ran
Luo, Xiangpeng
Zeng, Junbang
Li, Jiarui
Bialo, Izabela
Bluschke, Martin
Tang, Yang
Freyermuth, Jacob
Yu, Guichuan
Sutarto, Ronny
He, Feizhou
Weschke, Eugen
Tabis, Wojciech
Greven, Martin
Li, Yuan
Affiliation Peking Univ, Int Ctr Quantum Mat, Sch Phys, Beijing 100871, Peoples R China
Univ Minnesota, Sch Phys & Astron, Minneapolis, MN 55455 USA
AGH Univ Sci & Technol, Fac Phys & Appl Comp Sci, PL-30059 Krakow, Poland
TU Wien, Inst Solid State Phys, A-1040 Vienna, Austria
Max Planck Inst Solid State Res, D-70569 Stuttgart, Germany
Helmholtz Zentrum Berlin Mat & Energie, Wilhelm Conrad Rontgen Campus BESSY 2, D-12489 Berlin, Germany
Canadian Light Source, Saskatoon, SK S7N 2V3, Canada
Collaborat Innovat Ctr Quantum Matter, Beijing 100871, Peoples R China
Columbia Univ, Dept Phys, New York, NY 10027 USA
Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA
MIT, Dept Phys, Cambridge, MA 02139 USA
Keywords DENSITY-WAVE ORDER
PHASE-DIAGRAM
SCATTERING
FLUCTUATIONS
PSEUDOGAP
ENERGY
Issue Date 19-Jun-2020
Publisher PHYSICAL REVIEW B
Abstract Using resonant x-ray diffraction and Raman spectroscopy, we study charge correlations and lattice dynamics in two model cuprates, HgBa2CuO4+delta and HgBa2CaCu2O6+delta. We observe a maximum of the characteristic charge order temperature around the same hole concentration (p approximate to 0.09) in both compounds, and concomitant pronounced anomalies in the lattice dynamics that involve the motion of atoms in and/or adjacent to the CuO2 layers. These anomalies are already present at room temperature, and therefore precede the formation of the static charge correlations, and we attribute them to an instability of the CuO2 layers. Our finding implies that the charge order in the cuprates is an emergent phenomenon, driven by a fundamental variation in both lattice and electronic properties as a function of doping.
URI http://hdl.handle.net/20.500.11897/589931
ISSN 2469-9950
DOI 10.1103/PhysRevB.101.220509
Indexed SCI(E)
Appears in Collections: 量子材料科学中心

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