Title Observation of magnetoelastic effects in a quasi-one-dimensional spiral magnet
Authors Wang, Chong
Yu, Daiwei
Liu, Xiaoqiang
Chen, Rongyan
Du, Xinyu
Hu, Biaoyan
Wang, Lichen
Iida, Kazuki
Kamazawa, Kazuya
Wakimoto, Shuichi
Feng, Ji
Wang, Nanlin
Li, Yuan
Affiliation Peking Univ, Sch Phys, Int Ctr Quantum Mat, Beijing 100871, Peoples R China.
Comprehens Res Org Sci & Soc, Neutron Sci & Technol Ctr, Tokai, Ibaraki 3191106, Japan.
Japan Atom Energy Agcy, Mat Sci Res Ctr, Tokai, Ibaraki 3191195, Japan.
Collaborat Innovat Ctr Quantum Matter, Beijing 100871, Peoples R China.
Chinese Acad Sci, Beijing Inst Nanoenergy & Nanosyst, Beijing 100083, Peoples R China.
Peking Univ, Sch Phys, Int Ctr Quantum Mat, Beijing 100871, Peoples R China.
Feng, J (reprint author), Collaborat Innovat Ctr Quantum Matter, Beijing 100871, Peoples R China.
Keywords HIGH CRITICAL-TEMPERATURE
SPIN-PEIERLS TRANSITION
ANTIFERROMAGNETIC CHAIN
RAMAN-SCATTERING
NEEL STATE
CUGEO3
MULTIFERROICS
PHASE
LIGHT
DIMERIZATION
Issue Date 2017
Publisher PHYSICAL REVIEW B
Citation PHYSICAL REVIEW B.2017,96(8).
Abstract We present a systematic study of spin and lattice dynamics in the quasi-one-dimensional spiral magnet CuBr2, using Raman scattering in conjunction with infrared and neutron spectroscopy. Along with the development of spin correlations upon cooling, we observe a rich set of broad Raman bands at energies that correspond to phonon-dispersion energies near the one-dimensional magnetic wave vector. The low-energy bands further exhibit a distinct intensity maximum at the spiral magnetic ordering temperature. We attribute these unusual observations to two possible underlying mechanisms: (1) formation of hybrid spin-lattice excitations and/or (2) "quadrumerization" of the lattice caused by spin-singlet entanglement in competition with the spiral magnetism.
URI http://hdl.handle.net/20.500.11897/471560
ISSN 2469-9950
DOI 10.1103/PhysRevB.96.085111
Indexed SCI(E)
Appears in Collections: 物理学院

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