Title Third-order nonlinear optical properties of fullerene molecules
Authors Gong, Qihuang
Yang, Shaochen
Sun, Yuxing
Zou, Yinghua
Qiang, Di
Jing, Zhaoxia
Wu, Yongqing
Sun, Yiliang
Affiliation Peking Univ, Beijing, China
Issue Date 1993
Publisher guangxue xuebaoacta optica sinica
Citation Guangxue Xuebao/Acta Optica Sinica.1993,13,(6),496-499.
Abstract The third-order nonlinear optical properties of two kinds of fullerenes(molecules of C60 and C70) , which are solved in toluene, were studied through a degenerate four wave mixing process respectively. The third-order hyperpolarizabilities of C70 molecule and C60 molecule were measured to be 1.2??10-30 esu and 4.0??10-31 esu, corresponding to an estimated third-order optical susceptibility of 2.5??10-8 esu and 8.5??10-9 esu for solid-state materials, respectively. The origin of the large nonlinear optical response of fullerene family is explained successfully with the free electron model.
URI http://hdl.handle.net/20.500.11897/303065
ISSN 02532239
Indexed EI
Appears in Collections: 待认领

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