Title Epitaxial Heterostructures of Ultrathin Topological Insulator Nanoplate and Graphene
Authors Dang, Wenhui
Peng, Hailin
Li, Hui
Wang, Pu
Liu, Zhongfan
Affiliation Peking Univ, Ctr Nanochem, State Key Lab Struct Chem Unstable & Stable Speci, BNLMS,Coll Chem & Mol Engn, Beijing 100871, Peoples R China.
Keywords Topological insulator
graphene
Dirac materials
bismuth selenide
van der Waals epitaxy
SINGLE DIRAC CONE
ELECTRONIC-STRUCTURE
RAMAN-SPECTROSCOPY
BISMUTH TELLURIDE
NANOWIRES
NANORIBBONS
SURFACE
BI2TE3
BI2SE3
SELENIDE
Issue Date 2010
Publisher nano letters
Citation NANO LETTERS.2010,10,(8),2870-2876.
Abstract The authors present a van der Waals epitaxy of high-quality ultrathin nanoplates of topological insulator Bi2Se3 on a pristine graphene substrate using a simple vapor-phase deposition method. Sub-10-nm-thick nanoplates of layered Bi2Se3 with defined orientations can be epitaxially grown on a few-layer pristine graphene substrate. We show the evolution of Raman spectra with the number of Bi2Se3 layers on few-layer graphene. Bi2Se3 nanoplates with a thickness of three quintuple-layers (3-QL) exhibit the strongest Raman intensity. Strain effects in the Bi2Se3/graphene nanoplate heterostructures is also studied by Raman spectroscopy. 1-QL and 2-QL Bi2Se3 nanoplates experience tensile stress, consistent with compressive stress in single-layer and bilayer graphene substrates. Our results suggest an approach for the synthesis of epitaxial heterostructures that consist of an ultrathin topological insulator and graphene, which may be a new direction for electronic and spintronic applications.
URI http://hdl.handle.net/20.500.11897/150053
ISSN 1530-6984
DOI 10.1021/nl100938e
Indexed SCI(E)
PubMed
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